文章基本信息

标题：Unstable, Super Critical CO2–Water Displacement in Fine Grained Porous Media under Geologic Carbon Sequestration Conditions
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作者：R. Gooya ; A. Silvestri ; A. Moaddel 等
期刊名称：Scientific Reports
电子版ISSN：2045-2322
出版年度：2019
卷号：9
期号：1
页码：1-9
DOI：10.1038/s41598-019-47437-5
出版社：Springer Nature
摘要：In this study we investigated fluid displacement water with supercritical (sc) CO 2 in chalk under conditions close to those used for geologic CO 2 sequestration (GCS), to answer two main questions: How much volume is available for scCO 2 injection? And what is the main mechanism of displacement over a range of temperatures? Characterization of immiscible scCO 2 displacement, at the pore scale in the complex microstructure in chalk reservoirs, offers a pathway to better understand the macroscopic processes at the continuum scale. Fluid behavior was simulated by solving the Navier-Stokes equations, using finite-volume methods within a pore network. The pore network was extracted from a high resolution 3D image of chalk, obtained using X-ray nanotomography. Viscous fingering dominates scCO 2 infiltration and pores remain only partially saturated. The unstable front, developed with high capillary number, causes filling of pores aligned with the flow direction, reaching a maximum of 70% scCO 2 saturation. The saturation rate increases with temperature but the final saturation state is the same for all investigated temperatures. The higher the saturation rate, the higher the dynamic capillary pressure coefficient. A higher dynamic capillary pressure coefficient indicates that scCO 2 needs more time to reach capillary equilibrium in the porous medium.