文章基本信息

标题：Impulsive UV-pump/X-ray probe study of vibrational dynamics in glycine
本地全文：下载
作者：Riccardo Mincigrucci ; Markus Kowalewski ; Jérémy R. Rouxel 等
期刊名称：Scientific Reports
电子版ISSN：2045-2322
出版年度：2018
卷号：8
期号：1
页码：15466
DOI：10.1038/s41598-018-33607-4
语种：English
出版社：Springer Nature
摘要：We report an ab-initio study of a pump-probe experiment on the amino-acid glycine. We consider an UV pump followed by an X-ray probe tuned to carbon K-edge and study the vibronic structure of the core transition. The simulated experiment is feasible using existing free electron laser or high harmonic generation sources and thanks to the localization of the core orbitals posseses chemical selectivity. The present theory applies to other experimental schemes, including the use of a THz probe, available with present soft X-ray free electron lasers and/or high harmonic generation sources.