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标题：Regional non-CO 2 greenhouse gas fluxes inferred from atmospheric measurements in Ontario, Canada
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作者：F.R. Vogel ; M. Ishizawa ; E. Chan 等
期刊名称：Journal of Integrative Environmental Sciences
印刷版ISSN：1943-815X
电子版ISSN：1943-8168
出版年度：2012
卷号：9
期号：Supp 1
页码：41-55
DOI：10.1080/1943815X.2012.691884
出版社：Taylor & Francis
摘要：Abstract Independent verification of bottom-up greenhouse gas (GHG) emission inventories is crucial for a reliable reporting of Kyoto gases to the United Nations Framework Convention on Climate Change. Here, we use a pseudo-data experiment to test if our improved version of the well-known Radon tracer method (RTM) is able to quantitatively retrieve regional GHG fluxes. Using in-situ observations in Egbert, Canada, from 2006 to 2009 for the RTM, we derive night-time fluxes of CH 4 and N 2 O in southern Ontario. The N 2 O fluxes found have a inter-quartile range of 7.6–31.2 μgN 2 O/(m 2 h) with an overall mean of 24.4 ± 5.6 μgN 2 O/(m 2 h). Comparison with the EDGAR4.1 inventory revealed an underestimation by a factor of 1.7 ± 0.4 in the inventory, which is explainable by missing natural sources and a missing seasonal cycle in the inventory. Our RTM-based fluxes of CH 4 with a inter-quartiles range of 0.19–0.49 mgCH 4 /(m 2 h) and a mean of 0.36 ± 0.08 mgCH 4 /(m 2 h) lie significantly below the inventory-based estimates of 0.79 ± 0.06 mgCH 4 /(m 2 h). Using a Stochastic Time-Inverted Lagrangian Transport (STILT) model this difference can be attributed to an overestimation of CH 4 emissions in a specific region, the highly urbanized Greater Toronto Area. This study displays how the application of the RTM in future monitoring networks could help to assess high-resolution emission inventories.
关键词：non-CO2 greenhouse gases; regional flux estimate; Radon; top-down; urban emissions