文章基本信息

标题：Multidimensional photon correlation spectroscopy of cavity polaritons
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作者：Konstantin E. Dorfman ; Shaul Mukamel
期刊名称：Proceedings of the National Academy of Sciences
印刷版ISSN：0027-8424
电子版ISSN：1091-6490
出版年度：2018
卷号：115
期号：7
页码：1451-1456
DOI：10.1073/pnas.1719443115
语种：English
出版社：The National Academy of Sciences of the United States of America
摘要：The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency–resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes–Cummings model.
关键词：multidimensional spectroscopy ; photon correlation ; cavity polaritons