文章基本信息

标题：Induced Ferromagnetism at BiFeO₃/YBa₂Cu₃O₇ Interfaces
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作者：Jian-Xin Zhu ; Xiao-Dong Wen ; J. T. Haraldsen 等
期刊名称：Scientific Reports
电子版ISSN：2045-2322
出版年度：2014
卷号：4
DOI：10.1038/srep05368
出版社：Springer Nature
摘要：Transition metal oxides (TMOs) exhibit many emergent phenomena ranging from high-temperature superconductivity and giant magnetoresistance to magnetism and ferroelectricity. In addition, when TMOs are interfaced with each other, new functionalities can arise, which are absent in individual components. Here, we report results from first-principles calculations on the magnetism at the BiFeO₃/YBa₂Cu₃O₇ interfaces. By comparing the total energy for various magnetic spin configurations inside BiFeO₃, we are able to show that a metallic ferromagnetism is induced near the interface. We further develop an interface exchange-coupling model and place the extracted exchange coupling interaction strengths, from the first-principles calculations, into a resultant generic phase diagram. Our conclusion of interfacial ferromagnetism is confirmed by the presence of a hysteresis loop in field-dependent magnetization data. The emergence of interfacial ferromagnetism should have implications to electronic and transport properties.