文章基本信息

标题：Multidimensional four-wave mixing signals detected by quantum squeezed light
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作者：Konstantin Dorfman ; Shengshuai Liu ; Yanbo Lou 等
期刊名称：Proceedings of the National Academy of Sciences
印刷版ISSN：0027-8424
电子版ISSN：1091-6490
出版年度：2021
卷号：118
期号：33
DOI：10.1073/pnas.2105601118
语种：English
出版社：The National Academy of Sciences of the United States of America
摘要：Significance Quantum light and its statistics provide powerful tools for the study of properties of matter that are difficult to retrieve with classical light. Novel spectroscopic and sensing techniques based on quantum light sources can reveal information about complex material systems that is not accessible by varying the frequencies or time delays of classical light pulses. Here, based on a four-wave mixing process, we report an experimental study of the 2D quantum noise spectra of two-beam intensity difference squeezing. External noise erodes the resolution of classical measurements, while quantum signals remain intact. Our results pave the way for exploiting quantum correlations of squeezed light for spectroscopic applications. Four-wave mixing (FWM) of optical fields has been extensively used in quantum information processing, sensing, and memories. It also forms a basis for nonlinear spectroscopies such as transient grating, stimulated Raman, and photon echo where phase matching is used to select desired components of the third-order response of matter. Here we report an experimental study of the two-dimensional quantum noise intensity difference spectra of a pair of squeezed beams generated by FWM in hot Rb vapor. The measurement reveals details of the χ ( 3 ) susceptibility dressed by the strong pump field which induces an AC Stark shift, with higher spectral resolution compared to classical measurements of probe and conjugate beam intensities. We demonstrate how quantum correlations of squeezed light can be utilized as a spectroscopic tool which unlike their classical counterparts are robust to external noise.
关键词：enquantum spectroscopy;multidimensional spectroscopy;squeezed light