文章基本信息

标题：Enhanced second-harmonic generation in monolayer MoS2 on suspended metallic nanostructures by plasmonic resonances
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作者：Leng Qing ; Su Huanhuan ; Liu Jianqiang 等
期刊名称：Nanophotonics
印刷版ISSN：2192-8606
电子版ISSN：2192-8614
出版年度：2021
卷号：10
期号：7
页码：1871-1877
DOI：10.1515/nanoph-2021-0030
语种：English
出版社：Walter de Gruyter GmbH
摘要：Monolayer transition metal dichalcogenides (TMDs) possess large second-order nonlinear responses due to the broken inversion symmetry, which can extend their intriguing applications in nonlinear nanophotonics and optoelectronics. However, the atomic thickness of monolayer TMDs severely decreases the interaction length with free light with respect to bulk materials, leading to rather low second-harmonic generation (SHG) conversion efficiency. Here, we demonstrate a hybrid structure consisting of a monolayer MoS2 on a suspended perforated silver film, on which the SHG signal emitted from the monolayer MoS2 is enhanced by more than three orders of magnitude at room temperature. The pronounced SHG enhancement is attributed to the distinct electric field amplification nearby the nanoholes, which is induced by the symmetric surface plasmon polaritons (SPPs) existing in the ultrathin suspended silver grating. Our results reported here may establish the substrate-free engineering of nonlinear optical effects via plasmonic nanostructures on demand.